I used Handbrake 0.9.9 (64 bit) on OS X 10.8.4 with iTunes 11.0.4. I encoded the same movie using the AppleTV 2 preset and also the iPhone preset. It encoded successfully generating two .m4v files on my desktop. I couldn't "Add To Library" nor drag and drop into the library. They would play fine in QuickTime. Many hours of surfing later, the answer was simple: rename them to .mov files. Voila. In they went.